Topic 2.4: Chemical equilibria I

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2.4 (a) Dynamic chemical equilibrium
Chemical reactions which take place in both directions are called reversible reactions. Reactions like these however reach equilibrium. This is when chemical reactions are still occurring but the rates of the forward and reverse reactions are equal and so the concentration of each species remains constant. This type of system is said to be in dynamic equilibrium.
Example H2(g) + I2(g)  <=>2HI(g)          (A dynamic equilibrium).
The proportion of products to reactants in the equilibrium mixture is described as the equilibrium composition or as the position of equilibrium:

aP + bQ <=> cR + dS
If the conversion of P and Q into R and S is small the position of the equilibrium lies to the left.  If the equilibrium mixture is largely composed of R and S, the position of the equilibrium lies to the right.
The position of equilibrium is dependant on the equilibrium constant Kc and can also be altered by a change in external conditions such as concentration or pressure.  The equilibrium constant is only affected by a change in temperature.
Task 2.4a With reference to the reaction between hydrogen and iodine explain: (a) reversible reaction (b) equilibrium reaction (c) dynamic equilibrium (d) position of equilibrium (e) shifting the position of equilibrium to the right or left.

2.4 (b) Temperature, pressure and concentration and the position of equilibrium
Le Chatelier's principle states that when a reaction at equilibrium is subjected to a change in condition (temperature, pressure or concentration), the equilibrium composition/position alters to reduce the effect of the change.  Homogeneous equilibria describe those in which all of the substances are in the same phase e. g. all gases, all, liquids or all in aqueous solution.
When there is a change in concentration the position of an equilibrium changes. If a substance becomes more concentrated the position of the equilibrium shifts to reduce the concentration of that substance.  So for the reaction below:

4NH3(g) + 5O2(g) <=> 4NO(g) + 6H2O(g)    /\ H = -950kJmol-1
Increasing the concentration of ammonia causes the position of equilibrium to move to the right and for a bigger yield of product, nitrogen monoxide, to form.
Changes in pressure are important mainly in gaseous reactions.  Le Chatelier's principle can be applied to the formation of ammonia in the Haber process.

N2(g) + 3H2(g) <=> 2NH3(g)   /\ H = -92kJmol-1

When the pressure is increased the equilibrium shifts in the direction that tends to decrease the pressure. This is done by decreasing the number of molecules present, by moving the position of equilibrium from left to right.  A higher yield of the product ammonia results from the use of high pressure so typical plant operates at about 200 atmospheres pressure.  
For ammonia manufacture decreasing the temperature leads to a higher yield of ammonia because the reaction from left to right is exothermic and causes the temperature to rise again if ammonia is formed.  
watch animations of these effects
Task 2.4b  State and explain the effect of (a) increasing the temperature and (b) decreasing the pressure (c) decreasing the temperature (d) increasing the pressure on the following reactions:
2NO(g) + O2(g) = 2NO2(g) ;  DH = +57kJmol-1
2H2(g) + O2(g) = 2H2O(g) ;  DH = - 280kJmol-1
CH4(g) + H2O(g) = CO(g) + 3H2(g) ;  DH = + 40kJmol-1

2.4 (c) Catalyst and the position of equilibrium
Catalysts do not alter the equilibrium constant or the position of equilibrium. They do affect the time needed for the system to reach equilibrium.

2.4 (d) Temperature and optimum reaction conditions
In the Haber process a moderately high temperature of around 500oC is used to speed the rate at which equilibrium is reached.  This temperature is chosen in spite of the fact that a lower temperature gives a higher yield.  The manufacture of nitric acid involves 3 steps the first of which is the catalytic oxidation of ammonia to nitrogen monoxide.

4NH3(g) + 5O2(g) <=> 4NO(g) + 6H2O(g)    /\ H = -950kJmol-1
This reaction is run over a platinum gauze at 7 atmospheres and 900oC.  Low pressure favours the products as 9 molecules of reactant form 10 molecules of product.  However a higher pressure also increases the concentration of gas molecules of reactant molecules at the start and helps increase the yield of nitrogen monoxide.  Low temperature also favours products but a moderately high temperature is used so that equilibrium is reached quickly.
Task 2.4d Ethanol is made from ethene and water in the gas phase in an equilibrium reaction.  At 50 atmospheres the yield of ethanol is 30% at 320oC and 45% at 200oC.  At 80 atmospheres the yield of ethanol is 45% at 320oc AND 60% at 200oC.  Comment on the optimum conditions for this reaction.